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This question belongs to Competitive English Synonyms
Synonyms
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Synonym of UNTIE

Answer & Solution
Correct Answer: Option C
Unfold : open or spread out from a folded position.
Unchain : remove the chains fastening or securing (someone or something).
Undo : unfasten, untie, or loosen (something).
Unhinge : make (someone) mentally unbalanced.
Untie : undo or unfasten (something that is tied or tied up).

Synonym of Untie is Undo
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